Characterizing isotopic composition of post-accident/incident fallout
Posted: 27 Jan 2020, 07:14
Hi,
New here, an amateur from the west coast of the USA. I have a reasonably good layperson's understanding of radioactivity, isotopic decay chains, types of radiation, KeV spectra, principles of shielding, etc. Mostly with reference to nuclear safety concerns from reactor accidents (fuku / chernobyl / TMI / Windscale) and to possible nuclear war or terrorism. (Anything from isolated nuclear terrorism incident up to major nuclear exchange between major powers.)
At present I have a NukAlert ER rad detector. It's designed and tested to go all the way from single counts to 1 (one) full Sievert per hour without saturating.
In the unlikely event that I happen to be living in a place that ends up in the path of significant fallout from any sort of nuclear materials release, whether accidental or otherwise, I'm hoping to provide myself with usable data on the isotopic composition of fallout at my exact location. (Typically it's many days to weeks from the release incident until much solid info is released by government agencies, and even then it's only very general in nature.)
I've reviewed a good amount of the lower-cost (<$2000 USD) gamma spectroscopy equipment available for sale and have a general notion that a gam-spec setup could be very useful for characterizing post-accident/incident fallout composition. The main roadblock appears to be the low saturation threshold. Fallout particles or contaminated soil collected "shortly" after the incident (anything from hours to possibly months) is likely to be so active that it quickly saturates unshielded gam-spec equipment.
I assume that with a properly-calibrated reverse shielding setup (i.e. where the shield is configured to attenuate the sample material itself, rather than blocking out background radiation) I'd be able to take a pretty "hot" fallout sample and get usable data on its isotopic composition.
Assume for the purposes of this discussion that I would have already planned and prepared for relatively safe handling of said sample: For example: I emerge from a fallout shelter 48 hours post-incident and measure a radiation field averaging about 0.01 Sievert /hour. Low enough that I can afford to spend 5 minutes outdoors to collect a soil sample. I use a long-handled scoop to carefully put 10 mL's of soil into a clean ZipLoc sample bag, taking care to avoid even the slightest contam. of the outside of the bag. The sealed ZipLoc bag then goes into a small, portable, covered-top lead pig of perhaps no more than 20 kilos total weight, which itself had been set down temporarily on a piece of clean, disposable plastic sheeting. I take the covered lead pig & sample back into the shelter and attempt to perform gamma-spec measurements on it. (Assume also that I had already configured & tested my fallout shelter with a reasonably low BGR workstation area and that I had taken all necessary precautions to avoid tracking any soil or fallout back into the shelter, e.g. with proper donning & removal of tyvek bunny suit and shoe covers during sample collection, doing a careful radiation survey around the inside of the shelter with a rad meter to check for sources of stray emissions, etc.)
Is this a workable idea from a data-collection standpoint? I'm thinking that in principle it should be possible, either with just the portable lead pig itself or if need be with additional lead shielding, to attenuate the radiation to a level the gamma-spec equipment can handle. What I'm less certain about is whether the fallout would be so rich with a wide variety of isotopes that it might prove difficult or impossible to distinguish among the many different species in the mix.
Interested to hear comments & suggestions.
New here, an amateur from the west coast of the USA. I have a reasonably good layperson's understanding of radioactivity, isotopic decay chains, types of radiation, KeV spectra, principles of shielding, etc. Mostly with reference to nuclear safety concerns from reactor accidents (fuku / chernobyl / TMI / Windscale) and to possible nuclear war or terrorism. (Anything from isolated nuclear terrorism incident up to major nuclear exchange between major powers.)
At present I have a NukAlert ER rad detector. It's designed and tested to go all the way from single counts to 1 (one) full Sievert per hour without saturating.
In the unlikely event that I happen to be living in a place that ends up in the path of significant fallout from any sort of nuclear materials release, whether accidental or otherwise, I'm hoping to provide myself with usable data on the isotopic composition of fallout at my exact location. (Typically it's many days to weeks from the release incident until much solid info is released by government agencies, and even then it's only very general in nature.)
I've reviewed a good amount of the lower-cost (<$2000 USD) gamma spectroscopy equipment available for sale and have a general notion that a gam-spec setup could be very useful for characterizing post-accident/incident fallout composition. The main roadblock appears to be the low saturation threshold. Fallout particles or contaminated soil collected "shortly" after the incident (anything from hours to possibly months) is likely to be so active that it quickly saturates unshielded gam-spec equipment.
I assume that with a properly-calibrated reverse shielding setup (i.e. where the shield is configured to attenuate the sample material itself, rather than blocking out background radiation) I'd be able to take a pretty "hot" fallout sample and get usable data on its isotopic composition.
Assume for the purposes of this discussion that I would have already planned and prepared for relatively safe handling of said sample: For example: I emerge from a fallout shelter 48 hours post-incident and measure a radiation field averaging about 0.01 Sievert /hour. Low enough that I can afford to spend 5 minutes outdoors to collect a soil sample. I use a long-handled scoop to carefully put 10 mL's of soil into a clean ZipLoc sample bag, taking care to avoid even the slightest contam. of the outside of the bag. The sealed ZipLoc bag then goes into a small, portable, covered-top lead pig of perhaps no more than 20 kilos total weight, which itself had been set down temporarily on a piece of clean, disposable plastic sheeting. I take the covered lead pig & sample back into the shelter and attempt to perform gamma-spec measurements on it. (Assume also that I had already configured & tested my fallout shelter with a reasonably low BGR workstation area and that I had taken all necessary precautions to avoid tracking any soil or fallout back into the shelter, e.g. with proper donning & removal of tyvek bunny suit and shoe covers during sample collection, doing a careful radiation survey around the inside of the shelter with a rad meter to check for sources of stray emissions, etc.)
Is this a workable idea from a data-collection standpoint? I'm thinking that in principle it should be possible, either with just the portable lead pig itself or if need be with additional lead shielding, to attenuate the radiation to a level the gamma-spec equipment can handle. What I'm less certain about is whether the fallout would be so rich with a wide variety of isotopes that it might prove difficult or impossible to distinguish among the many different species in the mix.
Interested to hear comments & suggestions.